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Manganese catalysts for the oxidative condensation of methane with alkali and alkaline-earth metal salt additives Научная публикация

Журнал Bulletin of the Academy of Sciences of the USSR Division of Chemical Science
ISSN: 0568-5230 , E-ISSN: 2376-8444
Вых. Данные Год: 1987, Том: 36, Номер: 9, Страницы: 1975-1977 Страниц : 3 DOI: 10.1007/bf00958365
Авторы Minachev Kh.M. 1 , Usachev N.Ya. 1 , Khodakov Yu.S. 1 , Udut V.N. 1 , Makarov P.A. 1
Организации
1 N.D. Zelinskii Institute of Organic Chemistry, Academy of Sciences of the USSR, Moscow,
Реферат: The addition of acetates of alkali (Li, Na, K, and Cs) and alkaline-earth (Mg and Ca) metals affects the catalytic properties of Mn/SiO2 catalysts in the oxidation condensation of methane to give C2-hydrocarbons. The promotion effect of sodium salts depends on the nature of the salt anion. Greatest efficiency is found for the (Mn + NaCl)/SiO2 catalyst. At 800°C and methane/air mole ratio equal to 0.55, C2-hydrocarbons are formed on this catalyst with 25.8% yield and 77.5% selectivity; the ethylene content in the methane condensation products is 95%.
Библиографическая ссылка: Minachev K.M. , Usachev N.Y. , Khodakov Y.S. , Udut V.N. , Makarov P.A.
Manganese catalysts for the oxidative condensation of methane with alkali and alkaline-earth metal salt additives
Bulletin of the Academy of Sciences of the USSR Division of Chemical Science. 1987. V.36. N9. P.1975-1977. DOI: 10.1007/bf00958365 РИНЦ OpenAlex
Даты:
Поступила в редакцию: 2 дек. 1986 г.
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РИНЦ: 30924907
OpenAlex: W2068651454
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