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Kinetic Laws of Oxidation of para-tert-Butylcumene in the Presence of N-Hydroxyphthalimide Научная публикация

Журнал Kinetics and Catalysis
ISSN: 0023-1584 , E-ISSN: 1608-3210
Вых. Данные Год: 2023, Том: 64, Номер: 6, Страницы: 750–758 Страниц : DOI: 10.1134/S002315842306006X
Авторы Frolov A.S. 1 , Kurganova E.A. 1 , Sapunov V.N. 2 , Kozlovskii R.A. 2 , Koshel’ G.N. 1 , Yarkina E.M. 1
Организации
1 Yaroslavl State Technical University, Yaroslavl, 150023 Russia
2 Mendeleev University of Chemical Technology of Russia, Moscow, 125047 Russia
Реферат: The kinetics of the oxidation of para-tert-butylcumene to hydroperoxide by molecular oxygen in the presence of N-hydroxyphthalimide was studied. By analyzing the laws of the formation of hydroperoxide and byproducts, a mathematical model of the process was constructed, which adequately describes the changes in the concentrations of the main components of the reaction over time. The main role of N-hydroxyphthalimide is to convert peroxide radicals into the corresponding hydroperoxides, thereby reducing the yield of byproducts by decreasing the quadratic chain termination rate. Moreover, the formed N-hydroxyphthalimide radicals increase the rate of hydrocarbon oxidation. Thus, the use of N-hydroxyphthalimide in hydrocarbon oxidation processes results in an increase in the rate and selectivity of hydroperoxide formation.
Библиографическая ссылка: Frolov A.S. , Kurganova E.A. , Sapunov V.N. , Kozlovskii R.A. , Koshel’ G.N. , Yarkina E.M.
Kinetic Laws of Oxidation of para-tert-Butylcumene in the Presence of N-Hydroxyphthalimide
Kinetics and Catalysis. 2023. V.64. N6. P.750–758. DOI: 10.1134/S002315842306006X WOS Scopus РИНЦ CAPlusCA OpenAlex
Оригинальная версия: Фролов А.С. , Курганова Е.А. , Сапунов В.Н. , Козловский Р.А. , Кошель Г.Н. , Яркина Е.М.
Кинетические закономерности процесса окисления пара-трет-бутилкумола в присутствии N-гидроксифталимида
Кинетика и катализ. 2023. Т.64. №6. С.720-729. DOI: 10.31857/S0453881123060072 РИНЦ OpenAlex
Даты:
Поступила в редакцию: 8 февр. 2023 г.
Принята к публикации: 15 июн. 2023 г.
Опубликована online: 12 дек. 2023 г.
Идентификаторы БД:
Web of science: WOS:001122621800006
Scopus: 2-s2.0-85179683335
РИНЦ: 64673185
Chemical Abstracts: 2023:2603178
Chemical Abstracts (print): 185:361850
OpenAlex: W4389616648
Альметрики: