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Ruthenium Nanoparticles Supported on Nitrogen-Doped Carbon Nanofibers for the Catalytic Wet Air Oxidation of Phenol Научная публикация

Журнал Applied Catalysis B: Environmental
ISSN: 0926-3373
Вых. Данные Год: 2014, Том: 146, Номер: SI, Страницы: 177-185 Страниц : 9 DOI: 10.1016/j.apcatb.2013.03.017
Авторы Ayusheev Artemiy B. 1 , Taran Oxana P. 1 , Seryak Ivan A. 1 , Podyacheva Olga Yu. 1 , Descorme Claude 2 , Besson Mishele 2 , Kibis Lidiya S. 1 , Boronin Andrey I. 1,3 , Romanenko Anatoly I. 4 , Ismagilov Zinfer R. 1 , Parmon V. 1,3
Организации
1 Boreskov Institute of Catalysis, Siberian Branch of the Russian Academy of Sciences, 5 pr. Lavrentieva, 630090, Novosibirsk, Russia
2 Institut de recherches sur la catalyse et l’environnement de Lyon (IRCELYON), UMR 5256 CNRS - Université de Lyon, 2 Avenue Albert Einstein, 69626, Villeurbanne, France
3 Novosibirsk State University, 2 Pirogova st., 630090, Novosibirsk, Russia
4 Nikolaev Institute of Inorganic Chemistry, Siberian Branch of the Russian Academy of Sciences, 3 pr. Lavrentieva, 630090, Novosibirsk, Russia
Реферат: The effect of nitrogen content in N-doped carbon nanofibers (N-CNFs) on the catalytic activity of Ru/N-CNFs in the wet air oxidation of phenol has been studied. The N-CNFs, irrespective of nitrogen content and Sibunit, are shown to be low active. In the case of Ru-containing catalysts, nitrogen in N-CNFs was found to be responsible for both the increased activity and stability of the catalysts toward deactivation. The XPS showed the formation of carbon-oxygen structures with hydroxyl (carbonyl) end groups blocking ruthenium on the surface of the catalysts without nitrogen. For the catalysts with nitrogen, the ruthenium nanoparticles were not blocked in the course of the reaction and mainly the carboxyl (carbonate) surface groups were formed. The nature of this effect is discussed.
Библиографическая ссылка: Ayusheev A.B. , Taran O.P. , Seryak I.A. , Podyacheva O.Y. , Descorme C. , Besson M. , Kibis L.S. , Boronin A.I. , Romanenko A.I. , Ismagilov Z.R. , Parmon V.
Ruthenium Nanoparticles Supported on Nitrogen-Doped Carbon Nanofibers for the Catalytic Wet Air Oxidation of Phenol
Applied Catalysis B: Environmental. 2014. V.146. NSI. P.177-185. DOI: 10.1016/j.apcatb.2013.03.017 WOS Scopus РИНЦ CAPlusCA OpenAlex Sciact
Даты:
Поступила в редакцию: 30 окт. 2012 г.
Принята к публикации: 8 мар. 2013 г.
Опубликована online: 18 мар. 2013 г.
Опубликована в печати: 1 мар. 2014 г.
Идентификаторы БД:
Web of science: WOS:000327904000021
Scopus: 2-s2.0-84885485937
РИНЦ: 21860879
Chemical Abstracts: 2013:523233
Chemical Abstracts (print): 159:644896
OpenAlex: W2030228968
Sciact: 3675
Цитирование в БД:
БД Цитирований
Scopus 95
OpenAlex 94
Альметрики: