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A Kinetic Model of Standard Selective Catalytic Reduction of NO by NH3 on Two Sites Научная публикация

Журнал Reaction Kinetics, Mechanisms and Catalysis
ISSN: 1878-5190 , E-ISSN: 1878-5204
Вых. Данные Год: 2011, Том: 104, Номер: 2, Страницы: 267-272 Страниц : 6 DOI: 10.1007/s11144-011-0353-9
Авторы Zhdanov Vladimir P. 1,2
Организации
1 Competence Centre for Catalysis, Chalmers University of Technology, S-41296 Go¨teborg, Sweden
2 Boreskov Institute of Catalysis, Russian Academy of Sciences, Novosibirsk 630090, Russia
Реферат: Reduction of NO by NH3 in the presence of O2 may occur on single Fe or Cu atoms or dimers incorporated into the inner walls of zeolite. One of the likely schemes of this reaction implies the formation of N2 and H2O through the reaction of gas-phase NO and adsorbed NH3. The steady-state kinetics corresponding to this scheme was recently analyzed by the author assuming that the reaction runs on single metal atoms. In this work, the author presents a model including two metal atoms. Under the practically important conditions, the kinetics predicted by the one- and two-site models are demonstrated to be similar. In particular, both models allow one to interpret the apparent reaction orders observed experimentally.
Библиографическая ссылка: Zhdanov V.P.
A Kinetic Model of Standard Selective Catalytic Reduction of NO by NH3 on Two Sites
Reaction Kinetics, Mechanisms and Catalysis. 2011. V.104. N2. P.267-272. DOI: 10.1007/s11144-011-0353-9 WOS Scopus РИНЦ CAPlusCA OpenAlex Sciact
Даты:
Поступила в редакцию: 4 июн. 2011 г.
Принята к публикации: 15 июл. 2011 г.
Опубликована online: 2 авг. 2011 г.
Опубликована в печати: 1 дек. 2011 г.
Идентификаторы БД:
Web of science: WOS:000297169300003
Scopus: 2-s2.0-84877580048
РИНЦ: 20527946
Chemical Abstracts: 2011:1472992
Chemical Abstracts (print): 156:211143
OpenAlex: W4247426825
Sciact: 8101
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БД Цитирований
Scopus 3
OpenAlex 3
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